From Wikipedia, the free encyclopedia
Shevchenko BN350 nuclear fast reactor and desalination plant situated on the shore of the
Caspian Sea. The plant generated 135 MW
e and provided steam for an associated desalination plant. View of the interior of the reactor hall.
A
fast-neutron reactor or simply a
fast reactor is a category of
nuclear reactor in which the fission
chain reaction is sustained by
fast neutrons, as opposed to
thermal neutrons used in
thermal-neutron reactors. Such a reactor needs no
neutron moderator, but must use
fuel that is relatively rich in
fissile material when compared to that required for a
thermal reactor.
Introduction
Basic fission concepts
In order to sustain a fission
chain reaction,
the neutrons released in fission events have to react with other atoms
in the fuel. The chance of this occurring depends on the energy of the
neutron; most atoms will only undergo induced fission with high energy
neutrons, although a smaller number prefer much lower energies.
Natural uranium consists mostly of three
isotopes,
U-238,
U-235, and trace quantities of
U-234,
a decay product of U-238. U-238 accounts for roughly 99.3% of natural
uranium and undergoes fission only by neutrons with energies of 5 MeV or
greater, the so-called
fast neutrons[1].
About 0.7% of natural uranium is U-235, which undergoes fission by
neutrons of any energy, but particularly by lower energy neutrons. When
either of these isotopes undergoes fission they release neutrons with an
energy distribution peaking around 1 to 2 MeV. The flux of higher
energy fission neutrons (> 2 MeV) is too low to create sufficient
fission in U-238, and the flux of lower energy fission neutrons (< 2
MeV) is too low to do so easily in U-235
[2].
The common solution to this problem is to slow the neutron from these fast speeds using a
neutron moderator,
any substance which interacts with the neutrons and slows their speed.
The most common moderator is normal water, which slows the neutrons
through elastic scattering until the neutrons reach
thermal equilibrium
with the water. The key to reactor design is to carefully lay out the
fuel and water so the neutrons have time to slow enough to become highly
reactive with the U-235, but not so far as to allow them easy pathways
to escape the reactor core entirely.
Although U-238 will not undergo fission by the neutrons released in
fission, thermal neutrons can be captured by the nucleus to transmute
the atom into
Pu-239. Pu-239 has a
neutron cross section
very similar to that of U-235, and most of the atoms created this way
will undergo fission from the thermal neutrons. In most reactors this
accounts for as much as ⅓ of the energy being generated. Not all of the
Pu-239 is burned up during normal operation, and the leftover, along
with leftover U-238, can be separated out to be used in new fuel during
nuclear reprocessing.
Water is a common moderator for practical reasons, but has its
disadvantages. From a nuclear standpoint, the primary problem is that
water can absorb a neutron and remove it from the reaction. It does this
just enough that the amount of U-235 in natural ore is too low to
sustain the chain reaction; the neutrons lost through absorption in the
water and U-238, along with those lost to the environment, results in
too few left in the fuel. The most common solution to this problem is to
slightly concentrate the amount of U-235 in the fuel to produce
enriched uranium, with the leftover U-238 known as
depleted uranium. Other designs use different moderators, like
heavy water, that are much less likely to absorb neutrons, allowing them to run on unenriched fuel. In either case, the reactor's
neutron economy is based on
thermal neutrons.
Fast fission, breeders
Although
U-235 and Pu-239 are less sensitive to higher energy neutrons, they
still remain somewhat reactive well into the MeV area. If the fuel is
enriched, eventually a threshold will be reached where there are enough
fissile atoms in the fuel to maintain a chain reaction even with fast
neutrons.
The primary advantage is that by removing the moderator, the size of
the reactor can be greatly reduced, and to some extent the complexity.
This is commonly used for shipboard and submarine reactor systems, where
size and weight are major concerns. The downside to the fast reaction
is that fuel enrichment is an expensive process, so this is generally
not suitable for electrical generation or other roles where cost is more
important than size.
There is another advantage to the fast reaction that has led to
considerable development for civilian use. Fast reactors lack a
moderator, and thus lack one of the systems that remove neutrons from
the system. Those running on Pu-239 further increase the number of
neutrons, because its most common fission cycle gives off three neutrons
rather than the mix of two and three neutrons released from U-235. By
surrounding the reactor core with a moderator and then a
blanket
of U-238, those neutrons can be captured and used to breed more Pu-239.
This is the same reaction that occurs internally in conventional
designs, but in this case the blanket does not have to sustain a
reaction and thus can be made of natural uranium or even depleted
uranium.
Due to the surplus of neutrons from Pu-239 fission, the reactor will actually
breed
more Pu-239 than it consumes. The blanket material can then be
processed to extract the Pu-239 to replace the losses in the reactor,
and the surplus is then mixed with other fuel to produce
MOX fuel
that can be fed into conventional slow neutron reactors. A single fast
reactor can thereby feed several slow ones, greatly increasing the
amount of energy extracted from the natural uranium, from less than 1%
in a normal once-through cycle, to as much as 60% in the best fast
reactor cycles.
Given the limited stores of natural uranium ore, and the rate that
nuclear power was expected to take over baseload generation, through the
1960s and 70s fast breeder reactors were seen as the solution to the
world's energy needs. Using twice-through processing, a fast breeder
economy increases the fuel capacity of known ore deposits by as much as
100 times, meaning that even existing ore sources would last hundreds of
years. The disadvantage to this approach is that the breeder reactor
has to be fed highly enriched fuel, which is very expensive to produce.
Even though it breeds more fuel than it consumes, the resulting MOX is
still expensive. It was widely expected that this would still be below
the price of enriched uranium as demand increased and known resources
dwindled.
Through the 1970s, breeder designs were being widely experimented on,
especially in the USA, France and the USSR. However, this coincided
with a crash in uranium prices. The expected increased demand led mining
companies to build up new supply channels, which came online just as
the rate of reactor construction stalled in the mid-1970s. The resulting
oversupply caused fuel prices to decline from about US$40 per pound in
1980 to less than $20 by 1984. Breeders produced fuel that was much more
expensive, on the order of $100 to $160, and the few units that had
reached commercial operation proved to be economically disastrous.
Interest in breeder reactors were further muted by
Jimmy Carter's
April 1977 decision to defer construction of breeders in the US due to
proliferation concerns, and the terrible operating record of France's
Superphénix reactor.
Advantages
Fast neutron reactors can reduce the total radiotoxicity of nuclear waste, and dramatically reduce the waste's lifetime.
[8] They can also use all or almost all of the fuel in the waste. Fast neutrons have an advantage in the
transmutation of
nuclear waste. With fast neutrons, the ratio between
splitting and the
capture of
neutrons of
plutonium or
minor actinide
is often larger than when the neutrons are slower, at thermal or
near-thermal "epithermal" speeds. The transmuted even-numbered actinides
(e.g. Pu-240, Pu-242) split nearly as easily as odd-numbered actinides
in fast reactors. After they split, the
actinides
become a pair of "fission products." These elements have less total
radiotoxicity. Since disposal of the fission products is dominated by
the most radiotoxic
fission product,
cesium-137, which has a half life of 30.1 years,
[8]
the result is to reduce nuclear waste lifetimes from tens of millennia
(from transuranic isotopes) to a few centuries. The processes are not
perfect, but the remaining transuranics are reduced from a significant
problem to a tiny percentage of the total waste, because most
transuranics can be used as fuel.
- Fast reactors technically solve the "fuel shortage" argument against
uranium-fueled reactors without assuming unexplored reserves, or
extraction from dilute sources such as ordinary granite or the ocean.
They permit nuclear fuels to be bred from almost all the actinides,
including known, abundant sources of depleted uranium and thorium, and
light water reactor wastes. On average, more neutrons per fission are
produced from fissions caused by fast neutrons than from those caused by
thermal neutrons.
This results in a larger surplus of neutrons beyond those required to
sustain the chain reaction. These neutrons can be used to produce extra
fuel, or to transmute long half-life waste to less troublesome isotopes,
such as was done at the Phénix reactor in Marcoule in France, or some can be used for each purpose. Though conventional thermal reactors
also produce excess neutrons, fast reactors can produce enough of them
to breed more fuel than they consume. Such designs are known as fast breeder reactors.[citation needed]
Disadvantages
- Fast-neutron reactors are costly to build and operate, and are not
likely to be cost-competitive with thermal neutron reactors unless the
price of uranium increases dramatically.[9]
- Due to the low cross sections of most materials at high neutron energies, critical mass in a fast reactor is much higher than in a thermal reactor. In practice, this means significantly higher enrichment: >20% enrichment in a fast reactor compared to <5 a="" enrichment="" greater="" href="https://en.wikipedia.org/wiki/Nuclear_proliferation" in="" raises="" reactors.="" thermal="" this="" title="Nuclear proliferation" typical="">nuclear proliferation5>
and nuclear security issues.
[citation needed]
Sodium is often used as a coolant in fast reactors, because it does
not moderate neutron speeds much and has a high heat capacity. However,
it burns and foams in air. It has caused difficulties in reactors (e.g. USS Seawolf (SSN-575), Monju), although some sodium-cooled fast reactors have operated safely (notably the Superphénix and EBR-II for 30 years).[citation needed]
Since liquid metals other than lithium and beryllium have low
moderating ability, the primary interaction of neutrons with fast
reactor coolant is the (n,gamma) reaction, which induces radioactivity
in the coolant. Neutron irradiation activates a significant fraction of
coolant in high-power fast reactors, up to around a terabecquerel of
beta decays per kilogram of coolant in steady operation.[10]
Boiling in the coolant, e.g. in an accident, would reduce coolant
density and thus the absorption rate, such that the reactor has a
positive void coefficient, which is dangerous and undesirable from a safety and accident standpoint. This can be avoided with a gas cooled reactor,
since voids do not form in such a reactor during an accident; however,
activation in the coolant remains a problem. A helium-cooled reactor
would avoid this, since the elastic scattering and total cross sections
are approximately equal, i.e. there are very few (n,gamma) reactions in
the coolant and the low density of helium at typical operating
conditions means that the amount neutrons have few interactions with
coolant.[citation needed]
Nuclear reactor design
Coolant
Water, the most common
coolant in
thermal reactors, is generally not a feasible coolant for a fast reactor, because it acts as a
neutron moderator. However the
Generation IV reactor known as the
supercritical water reactor with decreased coolant density may reach a hard enough
neutron spectrum
to be considered a fast reactor. Breeding, which is the primary
advantage of fast over thermal reactors, may be accomplished with a
thermal, light-water cooled & moderated system using very high
enriched (~90%) uranium.
All current fast reactors are
liquid metal cooled reactors. The early
Clementine reactor used
mercury coolant and
plutonium metal fuel. Sodium-potassium alloy (
NaK) coolant is popular in test reactors due to its low
melting point.
In addition to its toxicity to humans, mercury has a high cross section
for the (n,gamma) reaction, causing activation in the coolant and
losing neutrons that could otherwise be absorbed in the fuel, which is
why it is no longer used or considered as a coolant in reactors. Molten
lead
cooling has been used in naval propulsion units as well as some other
prototype reactors. All large-scale fast reactors have used molten
sodium coolant.
Another proposed fast reactor is a
Molten Salt Reactor,
one in which the molten salt's moderating properties are insignificant.
This is typically achieved by replacing the light metal fluorides (e.g.
Lithium fluoride - LiF,
Beryllium fluoride - BeF
2) in the salt carrier with heavier metal chlorides (e.g.,
Potassium chloride - KCI,
Rubidium chloride - RbCl,
Zirconium chloride - ZrCl
4). Moltex Energy
[11] based in the UK proposes to build a fast neutron reactor called the
Stable Salt Reactor.
In this reactor design the nuclear fuel is dissolved in a molten salt.
The fuel salt is contained in stainless steel tubes similar to those use
in solid fuel reactors. The reactor is cooled using the natural
convection of another molten salt coolant. Moltex claims that their
design will be less expensive to build than a coal fired power plant and
can consume nuclear waste from conventional solid fuel reactors.
Gas-cooled fast reactors
have been the subject of research as well, as helium, the most commonly
proposed coolant in such a reactor, has small absorption and scattering
cross sections, thus preserving the fast neutron spectrum without
significant neutron absorption in the coolant.
[citation needed]
Nuclear fuel
In practice, sustaining a fission
chain reaction with
fast neutrons means using relatively highly
enriched uranium or
plutonium. The reason for this is that fissile reactions are favored at thermal energies, since the ratio between the Pu239
fission cross section and U238
absorption cross section
is ~100 in a thermal spectrum and 8 in a fast spectrum. Fission and
absorption cross sections are low for both Pu239 and U238 at high (fast)
energies, which means that fast neutrons are likelier to pass through
fuel without interacting than thermal neutrons; thus, more fissile
material is needed. Therefore it is impossible to build a fast reactor
using only
natural uranium fuel. However, it is possible to build a fast reactor that will
breed fuel (from
fertile material) by producing more fissile material than it consumes. After the initial fuel charge such a reactor can be refueled by
reprocessing.
Fission products can be replaced by adding natural or even depleted uranium with no further enrichment required. This is the concept of the
fast breeder reactor or FBR.
So far, most fast neutron reactors have used either
MOX (mixed oxide) or
metal alloy
fuel. Soviet fast neutron reactors have been using (high U-235
enriched) uranium fuel. The Indian prototype reactor has been using
uranium-carbide fuel.
While criticality at fast energies may be achieved with uranium
enriched to 5.5 weight percent Uranium-235, fast reactor designs have
often been proposed with enrichments in the range of 20 percent for a
variety of reasons, including core lifetime: If a fast reactor were
loaded with the minimal critical mass, then the reactor would become
subcritical after the first fission had occurred. Rather, an excess of
fuel is inserted with reactivity control mechanisms, such that the
reactivity control is inserted fully at the beginning of life to bring
the reactor from supercritical to critical; as the fuel is depleted, the
reactivity control is withdrawn to mitigate the negative reactivity
feedback from fuel depletion and fission product poisons. In a
fast breeder reactor,
the above applies, though the reactivity from fuel depletion is also
compensated by the breeding of either Uranium-233 or Plutonium-239 and
241 from Thorium 232 or Uranium 238, respectively.
Control
Like thermal reactors, fast neutron reactors are controlled by keeping the
criticality of the reactor reliant on
delayed neutrons, with gross control from neutron-absorbing control rods or blades.
They cannot, however, rely on changes to their moderators because there is no moderator. So
Doppler broadening in the moderator, which affects
thermal neutrons, does not work, nor does a negative
void coefficient of the moderator. Both techniques are very common in ordinary
light water reactors.
Doppler broadening from the molecular motion of the fuel, from its
heat, can provide rapid negative feedback. The molecular movement of the
fissionables themselves can tune the fuel's relative speed away from
the optimal neutron speed. Thermal expansion of the fuel itself can also
provide quick negative feedback. Small reactors such as those used in
submarines may use doppler broadening or thermal expansion of neutron
reflectors.
Shevchenko BN350 desalination unit. View of the only nuclear-heated desalination unit in the world
History
A 2008
IAEA proposal for a
Fast Reactor Knowledge Preservation System[12] notes that:
during the past 15 years there has been stagnation in the development
of fast reactors in the industrialized countries that were involved,
earlier, in intensive development of this area. All studies on fast
reactors have been stopped in countries such as Germany, Italy, the
United Kingdom and the United States of America and the only work being
carried out is related to the decommissioning of fast reactors. Many
specialists who were involved in the studies and development work in
this area in these countries have already retired or are close to
retirement. In countries such as France, Japan and the Russian
Federation that are still actively pursuing the evolution of fast
reactor technology, the situation is aggravated by the lack of young
scientists and engineers moving into this branch of nuclear power.
List of fast reactors
Decommissioned reactors
United States
- CLEMENTINE, the first fast reactor, built in 1946 at Los Alamos National Laboratory. Plutonium metal fuel, mercury coolant, power 25 kW thermal, used for research, especially as a fast neutron source.
- EBR-I at Idaho Falls, which in 1951 became the first reactor to generate significant amounts of electrical power. Decommissioned 1964.
- Fermi 1 near Detroit was a prototype fast breeder reactor that began operating in 1957 and shut down in 1972.
- EBR-II Prototype for the Integral Fast Reactor, 1965–1995?.
- SEFOR in Arkansas, a 20 MWt research reactor which operated from 1969 to 1972.
- Fast Flux Test Facility, 400 MWt, Operated flawlessly from 1982 to 1992, at Hanford Washington, now deactivated, liquid sodium is drained with argon backfill under care and maintenance.
Europe
- DFR (Dounreay Fast Reactor, 1959–1977, 14 MWe) and PFR (Prototype Fast Reactor, 1974–1994, 250 MWe), in Caithness, in the Highland area of Scotland.
- Rhapsodie in Cadarache, France, (20 then 40 MW) between 1967 and 1982.
- Superphénix, in France, 1200 MWe, closed in 1997 due to a political decision and very high costs of operation.
- Phénix,
1973, France, 233 MWe, restarted 2003 at 140 MWe for experiments on
transmutation of nuclear waste for six years, ceased power generation in
March 2009, though it will continue in test operation and to continue
research programs by CEA until the end of 2009. Stopped in 2010.
- KNK-II, Germany
USSR/Russia
- Small lead-cooled fast reactors used for naval propulsion, particularly by the Soviet Navy.
- BR-5 - research fast neutron reactor at the Institute of Physics and Energy in Obninsk. Years of operation 1959-2002.
- BN-350, constructed by the Soviet Union in Shevchenko (today's Aqtau) on the Caspian Sea, 130 MWe plus 80,000 tons of fresh water per day.
- IBR-2 - research fast neutron reactor at the Joint Institute of Nuclear Research in Dubna (near Moscow).
- BN-600
- sodium-cooled fast breeder reactor at the Beloyarsk Nuclear Power
Station. Provides 560 MW to the Middle Urals power grid. In operation
since 1980.
- BN-800
- sodium-cooled fast breeder reactor at the Beloyarsk Nuclear Power
Station. Designed to generate 880 MW of electrical power. Started
producing electricity in October, 2014. Achieved full power in August,
2016.
Asia
- Monju reactor, 300 MWe, in Japan.
was closed in 1995 following a serious sodium leak and fire. It was
restarted May 6, 2010 and in August 2010 another accident, involving
dropped machinery, shut down the reactor again. As of June 2011, the
reactor has only generated electricity for one hour since its first
testing two decades prior.
Never operated
Currently operating
- BN-600, 1981, Russia, 600 MWe, scheduled end of life 2010[13] but still in operation.[14]
- BN-800, Russia, testing began June 27, 2014,[15][16] estimated total power 880 MW. Achieved full power in August, 2016.
- BOR-60
- sodium-cooled reactor at the Research Institute of Atomic Reactors in
Dmitrovgrad. In operation since 1980.(experimental purposes)
- FBTR, 1985, India, 10.5 MWt (experimental purposes)
- China Experimental Fast Reactor, 65 MWt (experimental purposes), planned 2009, critical 2010[17]
Under repair
- Jōyō (常陽),
1977–1997 and 2004–2007, Japan, 140 MWt. Experimental reactor, operated
as an irradiation test facility. After an incident in 2007, the reactor
is suspended for repairing, recovery works were planned to be completed
in 2014.[18]
Under construction
- PFBR, Kalpakkam, India, 500 MWe.
- CFR-600, China, 600 MWe.
In design phase
- BN-1200, Russia, build starting after 2014,[19] operation in 2018–2020[20]
- Toshiba 4S being developed in Japan and was planned to be shipped to Galena, Alaska (USA) but progress is stalled (see Galena Nuclear Power Plant)
- KALIMER, 600 MWe, South Korea, projected 2030.[21]
KALIMER is a continuation of the sodium cooled, metallic fueled, fast
neutron reactor in a pool represented by the Advanced Burner Reactor
(2006), S-PRISM (1998-present), Integral Fast Reactor (1984-1994), and EBR-II (1965-1995).
- Generation IV reactor (Helium·Sodium·Lead cooled) US-proposed international effort, after 2030
- JSFR, Japan, project for a 1500 MWe reactor began in 1998, but without success.
- ASTRID, France, project for a 600 MWe sodium-cooled reactor. Planned experimental operation in 2020.[22]
- MACR,
1 MWe, USA/Mars, projected 2033. MACR (Mars Atmospherically Cooled
Reactor) is a gas-cooled (Carbon Dioxide coolant) fast neutron reactor
intended to provide power to the planned Mars colonies.
Planned
- Future FBR, India, 600 MWe, after 2025[23]